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Phys. , 1987, 91,724, and references therein. 11 S. H. Linn, C. L. Liao, C. Liao, J. M. Brom Jr and C. Y. Ng, Chem. Phys. , 1984,105,645. 12 G. Tanner, Diplomarbeit (University of Freiburg 1989). 13 H. , 1985, 156,305; Physics and Chemistry oJ Small Clusters, ed. P. Jena, B. K. N. Khann, NATO AS1 Series 158 (Plenum Press, New York,1987), p. 667. 14 H. Haberland, C. Ludewigt, H-G. Schindler and D. R. , 1985,156, 157; H. Haberland, in The Chemical Physics of Clusters, 107th Enrico Fermi School, ed.

The relative intensities of the two groups below and above n = 11 depend sensitively on expansion conditions, but the minimum is always present. The ion intensities in fig. 6 are given on a logarithmic scale to emphasize the exponential increase at low cluster masses. I5 This similarity strengthens the argument that small Hg clusters are purely van der Waals bound, in contrast to the conclusions of ref. (6). 8 states probed. As mentioned above, photoionisation measures the singlet component and electron impact at threshold the triplet component of the density of states.

J. F. Broer, Physica, 1942,9,591. J. P. Gordon, H. J. Zeiger, and C. H. Townes, Phys. , 1955,95,282L. G. Porter, Proc. R. Soc. London, Ser. A , 1950, 200, 284. Porter, Discuss. , 1950,9,60. Molecular Spectroscopy 60 37 SUBSTANCES O F SHORT LIFE T H E ABSORPTION SPECTROSCOPY OF SUBSTANCES OF SHORT LIFE BY GEORGEPORTER Received 17th July, 1950 The experimental methods available for the absorption spectroscopy of free radicals are critically discussed with special reference to flash photolysis and spectroscopy.

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